The Externally Driven Spin-Boson Model and its Application to Laser Control of Intramolecular Eletctron Transfer in a Polar Solvent

  1. Statement of the Mathematical Model and its Physical Motivation
  2. The Fermi Golden Rule for Short-time Dynamics of the Model: the Channel Picture of Photon-Assisted Electron Transfer.
  3. Master Equations for Long-time Dynamics of the Model: the Field-Driven NIBA Equations.
  4. Predictions of the Field-Driven NIBA for effects due to applied laser fields on:
    • Electron Transfer rates
    • Long-time Steady state Electronic Populations
    • Optical Absorption Spectra
    • Stimulated Emission

Back to program