AMOS Journal Club
Quantum structured attosecond excitation of matter
Quantum fluctuations play a central role in quantum optics, yet their influence on electronic dynamics at attosecond timescales remains largely unexplored. Transferring such fluctuations to an electronic wavefunction requires an XUV attosecond source that varies from shot to shot while preserving attosecond phase coherence. Recent studies have demonstrated that high-harmonic generation (HHG) driven or perturbed by bright squeezed vacuum (BSV) produces attosecond pulses that retain the statistical properties of the driving field [1–3]. BSV provides an extreme example of quantum-structured light: although its average electric field vanishes, its instantaneous field exhibits strong fluctuations, producing alternating periods of near-silence and intense noise bursts each optical cycle.
In this talk, I will present how we imprint quantum-origin fluctuations onto an excited electronic wave packet and follow their evolution using attosecond transient absorption (ATA). Attosecond pulses with inherited quantum statistics serve as a pump that initiates stochastic electronic coherence in helium. An IR dressing field then maps this coherence onto the ATA spectrum. We record the interference between the incident and generated fields versus the XUV-IR delay, on a shot-to-shot basis, capturing the evolution of their joint statistics. Leveraging the interferometric nature of ATA [4], we reconstruct the temporal evolution of the complex excitation with attosecond precision, revealing how quantum fluctuations propagate into and shape electronic coherence.
[1] A. Rasputnyi et al., Nat. Phys. (2024). [3] M. Even-Tzur et al., arXiv (2025).
[2] S. Lemieux et al., Nat. Photon. (2024). [4] M. Wu et al., J. Phys. B (2016).