Zoom: https://weizmann.zoom.us/j/96278790117?pwd=T1ZjaHlxQjlEQkFIbE12UDJCazNwZz09
Two-dimensional layered (van-der-Waals) heterostructures, made by stacking different monolayers of semiconducting transition-metal dichalcogenides, have been drawing much attention as versatile platforms for studying fundamental solid-state phenomena and for designing opto-electronic devices. Interlayer excitons, electron-hole pairs that bind to each other across the interlayer spacing in these heterostructures, hold promise as key tools for probing the interlayer interface structure, and for exploring many-body interactions(1). With long lifetimes, spin polarization, and electric tunability, interlayer excitons are also promising as flexible information carriers(2, 3). However, they were mostly studied through the scope of their visible light emission, missing essential properties such as their momentum-space image or their absorption strength, necessary for rigorous study of their many-body interactions and potential applications.
In this talk I will present our recent studies aimed at measuring such unknown interlayer exciton properties and their dependence on the heterostructure. I will show a new interlayer exciton in WSe2/MoS2 heterostructures which we discovered based on its light emission in infra-red wavelengths, rather than in the visible range(4). I will demonstrate its properties as inferred from its optical interrogation. Then, I will present the quantitative measurement of the elusive optical absorption spectrum of interlayer excitons using electric-field modulation spectroscopy, essential for coherent coupling of light to those excitons(5). Finally, I will reveal how time- and angle-resolved photoemission spectroscopy is used to image the interlayer exciton in momentum-space, yielding its size and binding energy, so far inaccessible through optics(5).
